Charge-density wave associated with higher-order Fermi-surface nesting in monolayer VS2
نویسندگان
چکیده
Abstract Fermi-surface (FS) nesting originating from Peierls’ idea of electronic instabilities in one-dimensional materials is a key concept to stabilize charge-density wave (CDW), whereas its applicability two-dimensional (2D) under intensive debate. Here we report unusual CDW associated with the higher-order FS monolayer 2D VS2. Angle-resolved photoemission spectroscopy and scanning tunneling microscopy uncovered stripe $$\sqrt {21} R10.9^\circ \times \sqrt 3 R30^\circ$$ 21 R 10 . 9 ∘ × 3 0 periodicity together an energy-gap opening on entire FS. We suggest that this involves FS-nesting vector 2 q twice larger than normal one ( ), as supported by anomalies calculated phonon dispersion susceptibility. The present results cooperation leads fully gapped state unlike case conventional single which produces partial gap, pointing intriguing mechanism transition.
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ژورنال
عنوان ژورنال: npj 2D materials and applications
سال: 2023
ISSN: ['2397-7132']
DOI: https://doi.org/10.1038/s41699-023-00395-z